X Files Vs Twin Peaks Vs Twilight Zone after Supernatural?

Hi all,

I've seen Supernatural a few times now, and looking for something to scratch that itch. These three are on top of my list, but asking for what show to watch now that fits the requirements I need !

Which one has the most horror, episodes that will get under your skin, and overall spook me out or make me think, and have a good sense of mystery?

Thanks all in advance.