Remove OneDrive Folder from Syncing

At one point we rolled out a GPO that automatically starting syncing a SharePoint site document library to workstations. We have since moved to Intune and over the last few months we have noticed that the once large (now massive) document library is slowing down machines and constantly syncing and indexing.

Is there a way with Intune or PS that I can get that folder to stop syncing on all machines and remove the directory?